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Multiple Rabi Splittings under Ultrastrong Vibrational Coupling

Research paper by Jino George, Thibault Chervy, Atef Shalabney, Eloïse Devaux, Hidefumi Hiura, Cyriaque Genet, Thomas W. Ebbesen

Indexed on: 22 Oct '16Published on: 06 Oct '16Published in: Physical review letters



Abstract

Author(s): Jino George, Thibault Chervy, Atef Shalabney, Eloïse Devaux, Hidefumi Hiura, Cyriaque Genet, and Thomas W. EbbesenFrom the high vibrational dipolar strength offered by molecular liquids, we demonstrate that a molecular vibration can be ultrastrongly coupled to multiple IR cavity modes, with Rabi splittings reaching 24% of the vibration frequencies. As a proof of the ultrastrong coupling regime, our experimental…[Phys. Rev. Lett. 117, 153601] Published Thu Oct 06, 2016